Time-dependent Hartree-Fock theory: finite-field technique for calculation of the Pockels and Kerr effects and generation of harmonics

M. M. Mestechkin, G. E. Whyman

Research output: Contribution to journalArticlepeer-review

15 Scopus citations

Abstract

A combined method for calculation of the optical hyperpolarizability dispersion in a static field based on the TDHF approximation and finite-difference technique is proposed and applied to twelve donor-acceptor substituted organic molecules with pronounced nonlinear properties and also to the carbon icosahedral cluster C60.

Original languageEnglish
Pages (from-to)144-148
Number of pages5
JournalChemical Physics Letters
Volume214
Issue number2
DOIs
StatePublished - 29 Oct 1993
Externally publishedYes

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